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Hannover 2010 – scientific programme

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UP: Fachverband Umweltphysik

UP 4: Remote Sensing

UP 4.6: Talk

Wednesday, March 10, 2010, 15:30–15:45, M 11

Evidence for Iodine monoxide in the Antarctic snowpack from spectrosocopic Measurements — •Udo Frieß1, Tim Deutschmann1, Ben Gilfedder2, Rolf Weller3, and Ulrich Platt11Institut für Umweltphysik, Universität Heidelberg — 2Institut für Umweltgeologie, TU-Braunschweig — 3Alfred Wegener Institut für Polar- und Meeresforschung, Bremerhaven

Recent ground-based and space borne observations suggest the presence of significant amounts of iodine monoxide in the boundary layer of Antarctica, which are expected to have an impact on the ozone budget and might contribute to the formation of new airborne particles. So far, the source of these iodine radicals has been unknown.

Here we present long-term measurements of iodine monoxide at the German Antarctic research station Neumayer, which indicate that the snowpack is the main source for iodine radicals. The measurements have been performed using multi-axis differential optical absorption spectroscopy (MAX-DOAS). Using a coupled atmosphere - snowpack radiative transfer model, the comparison of the signals observed from scattered skylight and from light reflected by the snowpack yields several ppb of iodine monoxide in the upper layers of the sunlit snowpack throughout the year. Snow pit samples from Neumayer Station contain up to 700 ng/l of total iodine, representing a sufficient reservoir for these extraordinarily high IO concentrations.

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