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Regensburg 2016 – scientific programme

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O: Fachverband Oberflächenphysik

O 88: Frontiers of Electronic Structure Theory: Focus on Topology and Transport V

O 88.9: Talk

Thursday, March 10, 2016, 17:00–17:15, H24

Exciton dispersion in layered and 2D systems — •Francesco Sottile1,2, Giorgia Fugallo1,2, Pierluigi Cudazzo1,2, and Matteo Gatti1,2,31Laboratoire des Solides Irradiés, École Polytechnique, CNRS, CEA-IRAMIS, Université Paris-Saclay, F-91128 Palaiseau, France — 2European Theoretical Spectroscopy Facility — 3Synchrotron SOLEIL, L'Orme des Merisiers, Saint-Aubin, Boîte Postale 48, F-91192 Gif-sur-Yvette, France

The study of the exciton dispersion is of paramount importance for all applications involving light harvesting, beside providing fundamental knowledge about exciton mobility and migration. Using state-of-the-art ab initio many-body approach, like the Bethe-Salpeter equation [1], we present a first principle study of exciton dispersions in layered materials and 2D systems. Results for the former systems (on the prototypical hBN and MoS2) have been recently confirmed by experiments carried out at the Synchrotron ESRF [2]. For the latter (2D) systems we investigate exciton dispersion in graphane and hBN. From our results we provide a general picture of the mechanisms governing the dispersion of neutral excitations in 2D systems, and of the role played by the confinement of the electronic charge in setting the exciton binding energy. In particular we found that due to the strongly reduced screening of the Coulomb interaction in low- dimensional materials, the binding energy of both Wannier and Frenkel excitons in the optical spectra is large and comparable in size[3]. [1] M. Gatti et al., Phys. Rev. B 88, 155113 (2013) [2] G. Fugallo et al. Phys. Rev. B 92, 165122 (2015) [3] P. Cudazzo et al. submitted to Phys. Rev. Lett.

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