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Regensburg 2019 – wissenschaftliches Programm

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TT: Fachverband Tiefe Temperaturen

TT 50: Poster Session: Correlated Electrons 2

TT 50.11: Poster

Mittwoch, 3. April 2019, 15:00–18:30, Poster D

Crystal growth and characterization of the frustrated spin systems Cs2−xRbxCuCl4 — •Sarah Krebber, Christian Klein, and Cornelius Krellner — Physikalisches Institut, Goethe-Universität Frankfurt am Main, Max-von-Laue-Straße 1, D-60438 Frankfurt am Main-

Crystals of the antiferromagnetic insulator Cs2CuCl4 and the substitution series (Cs2−xRbx)CuCl4 (x = 0.1, 0.2) were grown by vertical Bridgman method. The controlled substitution of cesium atoms with the smaller rubidium, causes chemical pressure on the crystal lattice [1]. The essential magnetic units in these systems are Jahn-Teller distorted (CuCl4) tetrahedra, which are arranged in layers separated by the alkali atoms. These layers form a triangular lattice of localized Cu2+ spins, where the spins interact through exchange couplings. The resulting geometric frustration leads to quantum spin-liquid properties at low temperatures [2].

In addition to the growth and characterization of (Cs2−xRbx)CuCl4, we discuss the structural changes in the lattice parameters and the magnetic behavior of the substituted system in comparison to the well understood parent compound Cs2CuCl4.
H. T. Witteveen, D. L. Jongejan and V. Brandwijk, Mater. Res. Bull. 9, 345 (1974)
O. A. Starykh, H. Katsura, and L. Balents, Phys. Rev. B 82, 014421 (2010)

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