Regensburg 2022 – scientific programme

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CPP: Fachverband Chemische Physik und Polymerphysik

CPP 10: 2D Materials 2 (joint session HL/CPP/DS)

CPP 10.2: Talk

Monday, September 5, 2022, 15:15–15:30, H36

Concept of an all-optical THz near-field microscope for flakes of 2D materials — •Ahmad-Reza Etemadi, Sebastian Matschy, Ahana Bhattacharya, and Martin Mittendorff — Department of physics, University of Duisburg-Essen, 47057 Duisburg, Germany

While THz spectroscopy is an excellent tool to investigate the free charge carriers in many semiconducting materials, the long-wavelength is an inherent feature linked to a large spot size in the millimeter range, and thus large samples are required. Small flakes of two-dimensional materials exfoliated from bulk crystals are usually much smaller than the spot size of a conventional THz spectrometer. The direct detection of the THz signal in the vicinity of the flake gains the phase and amplitude information with a higher spatial resolution. This is accessible by placing the sample directly on top of an electro-optic crystal. Sampling the THz field at the flake position gives access to the complex conductivity and thus the carrier density as well as the carrier mobility. A frequency-doubled fiber laser with a pulse duration of about 80 fs at 780 nm is exploited to generate and sample the THz field. GaSe, and ZnTe are employed as electro-optic crystals. Here we present the current state of the near-field microscope and the first measurements of the spatial resolution. The experimental results are accompanied by rigorous modeling of the THz propagation within the electro-optic crystal.