Dresden 2011 – wissenschaftliches Programm
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MO: Fachverband Molekülphysik
MO 12: Femtosecond Spectroscopy III
MO 12.3: Vortrag
Mittwoch, 16. März 2011, 11:00–11:15, TOE 317
Femtosecond RIXS on liquid jets and first results from LCLS — Philippe Wernet1, •Kristjan Kunnus1, Martin Beye1, Simon Schreck1, Edlira Suljoti1, Christian Weniger1, Christian Kalus1, Kerstin Kalus1, Alexander Föhlisch1, Ivan Rajkovic2, Sebastian Grübel2, Wilson Quevedo2, Mirko Scholz2, Simone Techert2, Brian Kennedy3, Franz Hennies3, Dennis Nordlund4, Robert Hartsock5, Wenkai Zhang5, Kelly Gaffney5, Josh Turner6, Bill Schlotter6, Ida Joseffson7, and Michael Odelius7 — 1Institute for Methods and Instrumentation for Synchrotron Radiation Research, Helmholtz-Zentrum Berlin — 2Max-Planck-Institut für Biophysikalische Chemie — 3MAX-lab — 4SSRL, SLAC National Accelerator Laboratory — 5PULSE, SLAC National Accelerator Laboratory — 6LCLS, SLAC National Accelerator Laboratory — 7Stockholm University
We developed a set up for femtosecond time resolved resonant inelastic soft x-ray scattering (RIXS) on liquid jets in vacuum. This allows for complete probing of occupied and unoccupied valence states of molecules in real-time during chemical reactions in solutions. Results from the first experiments at the Linac Coherent Light Source (LCLS) on the photodissociation of Fe(CO)5 molecules in ethanol will be presented together with complementary results from the synchrotron radiation source BESSYII at the Helmholtz-Zentrum Berlin.