Berlin 2018 – wissenschaftliches Programm

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CPP: Fachverband Chemische Physik und Polymerphysik

CPP 33: Poster Session III

CPP 33.27: Poster

Dienstag, 13. März 2018, 14:00–16:00, Poster C

Spheroidal and conical shapes of ferrofluid-filled capsules in magnetic fields — •Christian Wischnewski and Jan Kierfeld — Department of Physics, Technische Universität Dortmund, 44221 Dortmund, Germany

We investigate the deformation of soft spherical elastic capsules filled with a ferrofluid in external uniform magnetic fields at fixed volume by a combination of numerical and analytical approaches. We develop a numerical iterative solution strategy based on nonlinear elastic shape equations to calculate the stretched capsule shape numerically and a coupled finite element and boundary element method to solve the corresponding magnetostatic problem, and employ different analytical approximations. The observed deformation behavior is qualitatively similar to the deformation of ferrofluid droplets in uniform magnetic fields. Homogeneous magnetic fields elongate the capsule, and a discontinuous shape transition from a spheroidal shape to a conical shape takes place at a critical field strength. We investigate how capsule elasticity modifies this hysteretic shape transition and show that conical capsule shapes are possible but involve diverging stretch factors at the tips, which gives rise to rupture for real capsule materials. At small fields capsules remain spheroidal, and we characterize the deformation of spheroidal capsules both analytically and numerically. Our results can be helpful in order to quantitatively determine capsule or ferrofluid material properties from magnetic deformation experiments. All results also apply to elastic capsules filled with a dielectric liquid in an external uniform electric field.