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Berlin 2018 – wissenschaftliches Programm

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CPP: Fachverband Chemische Physik und Polymerphysik

CPP 64: Nanostructures, Nanostructuring and Nanosized Soft Matter II

CPP 64.7: Vortrag

Donnerstag, 15. März 2018, 11:15–11:30, PC 203

Time resolved analysis of a Brownian motor — •Christian Schwemmer1, Stefan Fringes1,2, Urs Dürig1,3, and Armin Knoll11IBM Research - Zurich, Switzerland — 2Institute of Physical Chemistry, University of Zurich, Switzerland — 3SwissLitho AG, Zurich, Switzerland

Artificial Brownian motors mimic the mechanism behind intracellular transport in nature [1] and enable a controlled transport of particles in a fluid [2]. In our implementation, we use a novel approach based on geometry induced trapping [3] to define a ratchet shaped potential landscape inside a nanofluidic slit. By applying a zero-mean AC electric field across the slit, we observed transport of 60 nm gold nano particles at drift speeds of 50 µm/s. The high temporal resolution of our experimental setup allowed us to measure the probability density in-situ and its temporal evolution with sub millisecond resolution. We observed current reversal at 250 Hz, an effect predicted more than 20 years ago [4], illustrating the nonlinear character of the motor. Comparison with a parameter-free theoretical model based on the Fokker-Planck equation shows excellent agreement. Using the model we traced the origin of the current reversal to the asymmetric, almost static probability density distribution at high frequencies, which leads to a faster increase of the backward current after switching the field direction.
[1] Vale et al., Science, 288, 88, (2000)
Hänggi et al., Rev. Mod. Phys, 81, 387, (2009)
Krishnan et al., Nature, 467, 692, (2010)
Bartussek et al., Europhysics Letters, 28, 459, (1994)

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