Berlin 2018 – wissenschaftliches Programm
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TT: Fachverband Tiefe Temperaturen
TT 55: Multiferroic Oxide Thin Films and Heterostructures I (joint session KFM/TT/MA)
TT 55.2: Vortrag
Mittwoch, 14. März 2018, 10:00–10:15, EMH 225
Structure and Magnetism of the Co/PZT/LSMO Interface — •Holger Meyerheim1, Arthur Ernst2, Katayoon Mohseni1, Andrey Polyakov1, Nathalie Jedrecy3, Andy Quindeau1, Victor Antonov1, Manuel Valvidares4, Hari Vasili4, and Pierluigi Gargiani4 — 1MPI f. Mikrostrukturphysik, D-06120 Halle — 2Inst. für Th. Physik, JKU, A-4040 Linz, Austria — 3INSP, UPMC-Sorbonne Univ., 75005 Paris, France — 4Alba, 08290 Cerdanyola del Vallés, Spain
Using surface x-ray diffraction, x-ray absorption fine structure and x-ray circular dichroism (XMCD) experiments we have studied the geometric and magnetic properties of the Co/Pb(Ti0.8Zr0.2)O3 interface. Co deposition in submonolayer amounts on the 2 unit cells thick (Ti,Zr)O2 terminated Pb (Ti0.8Zr0.2)O3 (PZT) layer leads to the formation of a perovskite type structure with Co-O distances of approximately 2.0 Å (octahedral) and 2.8 Å (cubic) in addition to a metallic Co-Co correlation near 2.4 Å. Co-L2,3-XMCD spectra also reveal different Co environments, especially two Co-O contributions (A) and (B) related to the octahedral coordination (m=2.69µB) and the cubic coordination (m=2.33 µB). The XMCD analysis also evidences an anti-FM oriented induced moment at the PZT top layer Ti site (m=-0.005µB) related to the negative tunneling electro resistance effect. This result supports the "hybridization model" suggested by D.Pantel et al., Nat. Mat. 11, 289 (2012).
Support by SFB 762 (TP A5) is acknowledged. We thank E. Fonda (Samba at Soleil) and the ALBA staff for help during the experiments.