SAMOP 2021 – wissenschaftliches Programm

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A: Fachverband Atomphysik

A 3: Attosecond physics / Interaction with VUV and X-ray light

A 3.4: Hauptvortrag

Dienstag, 21. September 2021, 12:15–12:45, H1

Control of complex Fano resonances by shaped laser pulses — Camilo Granados, Nicola Mayer, Evgenii Ikonnikov, Misha Ivanov, and •Oleg Kornilov — Max-Born-Institute, Berlin

Ultrafast pulsed lasers and high-order harmonic generation have opened access to time-dependent studies in the extreme ultriviolet (XUV) photon energy range. Excited states accessible in the XUV region often have a complex character combining several coupled electronic states, such as multi-state Fano resonances, and undergo ultrafast relaxation dynamics via autoionization, dissociation or relaxation at conical intersections. Recently we investigated dynamics of the complex excited molecular states using time-resolved photoelectron [1,2] and photoion [3] spectroscopy with wavelength-selected XUV pulses. In this contribution we explore how these dynamics can be controlled by temporal and frequency shaping of the near-infrared pulses used to probe the relaxation dynamics induce by XUV.

[1] M. Eckstein et al., Phys. Rev. Lett. 116, 163003 (2016). [2] M. Eckstein et al., Faraday Discuss. 194, 509 (2016). [3] G. Reitsma et al., J. Phys. Chem. A 123, 3068 (2019).