Regensburg 2013 – wissenschaftliches Programm

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DS: Fachverband Dünne Schichten

DS 29: Focus Session: Organic Materials for Spintronics: From Spinterface to Devices (jointly with HL, MA, O)

DS 29.6: Topical Talk

Donnerstag, 14. März 2013, 12:15–12:45, H32

Spinterfaces as microscopic spin traps — •Mirko Cinchetti — Department of Physics and Research Center OPTIMAS, University of Kaiserslautern, Kaiserslautern, Germany

Interfaces between ferromagnetic materials and organic semiconductors - also known as spinterfaces - constitute an incredibly rich playground in the field of spintronics. For example, spinterfaces have the potential to be implemented as tunable spin filters, which will pave the way to a whole new class of advanced, i.e., actively controlled spintronics devices. The progress in the field of spinterface science depends thus critically on elucidating the still unexplored spin-dependent carrier dynamics at such hybrid interfaces.

We use time-resolved two-photon photoemission to optically pump and probe a hybrid electronic state forming at the prototypical spinterface between cobalt and the organometallic complex tris(8-hydroxyquinolinato)aluminium (Alq3). We generate a transient spin polarization in the hybrid interface state, and follow its behavior in four dimensions: energy, time, spin and momentum. We find that electrons are confined at the Co-Alq3 interface for times in the range of 0.5-1 ps, and that the confining potential is strongly spin dependent. Such spin-dependent trapping behavior elucidates the fundamental microscopic origin of the spin-filtering properties at spinterfaces, which is important for the design of next-generation spintronics devices based on tunable organic spin filters.