Regensburg 2022 – wissenschaftliches Programm

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CPP: Fachverband Chemische Physik und Polymerphysik

CPP 10: 2D Materials 2 (joint session HL/CPP/DS)

CPP 10.7: Vortrag

Montag, 5. September 2022, 16:45–17:00, H36

Pump probe signatures of interlayer excitons in TMDC heterostructures — •Henry Mittenzwey, Manuel Katzer, Andreas Knorr, and Malte Selig — Institut für Theoretische Physik, Nichtlineare Optik und Quantenelektronik, Technische Universität Berlin, Hardenbergstr. 36, 10623 Berlin, Germany

TMDC heterobilayers are promising candidates for novel optoelectronic applications, since they exhibit long-lived excitonic states with spatially separated electrons and holes located in different layers. The relaxation dynamics of these interlayer excitons and their interplay with intralayer excitons are still under investigation.

Here, we present a microscopic description for the phonon and tunneling induced formation and relaxation of intra- and interlayer excitons in a MoSe₂/WSe₂ stack. Based on the microscopic dynamics we calculate the pump probe signal for intra- and interlayer transition and their population dynamics including hot exciton bottleneck effects.